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Development of Dissolving Pulp from Phyllostachys pubescens Stem by Prehydrolysis Soda Cooking with 2-Methylanthraquinone

CHEM, Mouylin 筑波大学 DOI:10.15068/0002006179

2023.01.17

概要

Bamboo grows mostly in the tropics. It is also found in the subtropical and temperate zones of all continents excluding Europe. Further, it belongs to a group of large woody grasses. There are 1250 species within the 75 genera of bamboo, and most grow rapidly, attaining stand maturity in five years (Scurlock et al., 2000; Sugesty et al., 2015). Bamboo is grown in India, Myanmar, Thailand, Indonesia, China, Japan, the Philippines, Australia, South Africa, South America, and southern North America. Bamboo has many utilities in Asian countries, such as in manufacturing writing instruments, furniture, building materials, weaving materials, household utensils, and agricultural tools. In addition, bamboo is a raw material used in the making of paper, musical instruments, religious articles, medicine, weapons, and other items (Yunnan et al., 1996). Phyllostachys pubescens is originally from China, and its plantations cover an area of 20,000 km2, which accounts for 60% of the total area covered by bamboo in China. It was introduced to Japan around the 1750s. The species has been used as a source of both poles and edible shoots in South-East Asia, and the optimal temperature for its growth is approximately 13–20°C (Qiu et al., 1992).

Bamboo is a non-wood raw material alternative (long fiber) for producing dissolving pulp and is available in large quantities and diverse types (Sugesty et al., 2015). Cellulose, hemicellulose, and lignin are the main components of plant biomass. Cellulose is composed of D-glucose units bond by β-1,4,-glucosidic bonds. Cellulose with a degree of polymerization ≥ 10,000 is arranged in a microfibril structure. The hydrogen bonds in the cellulose structure provide tensile strength, are insoluble in most solvents, and are resistant to microbial degradation (Jørgensen et al., 2007). Hemicelluloses are heterogenous polymers that form different polymers of pentoses, including xylose and arabinose; hexoses, including glucose, mannose, and galactose; and sugar acids. Hemicelluloses can form side chains and exhibit some degree of acetylation when the degree of polymerization is < 200 (Jørgensen et al., 2007; Lau, 2012; Saha, 2003). Lignin is a large molecular structure composed of cross-linked polymers of phenolic monomers, including coniferyl alcohol, coumaryl alcohol, and sinapyl alcohol (Jørgensen et al., 2007). The largest component of the plant cell wall is cellulose, accounting for 35–50 wt% of plant dry mass, with hemicellulose accounting for 20–25 wt% and lignin for 10– 25 wt% (Saha, 2003). As Figure 1-1 shows, all lignocellulosic materials contain three main components: cellulose, hemicellulose, and lignin. However, the processes of extracting the components vary, which is taken into account in the type of cooking reagents adopted.

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Wu, C., Zhou, S., Zhao, C., Wang, D., 2014. Improved reactivity of bamboo dissolving pulp for the viscose process: Post-treatment with beating. BioResources. 9(2), 3449–3455. doi:10.15376/biores.9.2.3449-3455

Yuan, Z., Wen, Y., Kapu, N.S., Beatson, R., Mark Martinez, D., 2017. A biorefinery scheme to fractionate bamboo into high-grade dissolving pulp and ethanol. Biotechnol Biofuels. 10(1), 1–16. doi:10.1186/s13068-017-0723-2

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