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Record of ³H and ³⁶Cl from the Fukushima nuclear accident recovered from soil water in the unsaturated zone at Koriyama

Ohta, Tomoko Fifield, L. Keith Palcsu, László Tims, Stephen G. Pavetich, Stefan Mahara, Yasunori 京都大学 DOI:10.1038/s41598-023-46853-y

2023.11.11

概要

The opportunity to measure the concentrations of ³H and ³⁶Cl released by the Fukushima nuclear accident in 2011 directly in rain was lost in the early stage of the accident. We have, however, been able to reconstruct the deposition record of atmospheric ³H and ³⁶Cl following the accident using a bore hole that was drilled in 2014 at Koriyama at a distance of 60 km from the accident. The contributions of ³H and ³⁶Cl from the accident are 1.4 × 10¹³ and 2.0 × 10¹² atoms m⁻² respectively at this site. Very high concentrations of both ³H (46 Bq L⁻¹) and ³⁶Cl (3.36 × 10¹¹ atoms L⁻¹) were found in the unsaturated soil at depths between 300 and 350 cm. From these, conservative estimates for the ³H and ³⁶Cl concentrations in the precipitation in the ~ 6 weeks following the accident were 607 Bq L⁻¹ and 4.74 × 10¹⁰ atoms L⁻¹, respectively. A second hole drilled in 2016 showed that ³H concentrations in the unsaturated soil and shallow groundwater had returned to close to natural levels, although the ³⁶Cl concentrations were still significantly elevated above natural levels.

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Acknowledgements

This work was supported by JSPS Grants-in-Aid for Scientific Research (Kakenhi Grant Numbers, 24686098,

17K07024, 20H02674), Ichimura Foundation for New Technology and YESSA (Yanmar shigenjunkan zaidan).

We are deeply grateful to Dr. Leonard I. Wassenaar and Takuya Matsumoto, the IAEA and ATOMIKI staff for

their technical support and Prof. Tamotsu Kozaki, Hokkaido University, for the financial support for the collection of the sediment cores in Fukushima in 2016, and Central Research Institute of Electric Power Industry for

financial support for drilling of observation well in 2019. The Heavy Ion Accelerator Facility (HIAF) at ANU is

supported by the National Collaborative Research Infrastructure Strategy (NCRIS) of the Australian Government.

Author contributions

T.O. and Y.M. developed the original idea of the analyses presented in the manuscript and designed the field

study. Field data were collected by T.O. and Y.M. Laboratory analyses were performed by T.O., Y.M., L.P., and

K.F., S.T., S.P. The manuscript was written by T.O. and Y. M., with contributions from all coauthors.

Competing interests The authors declare no competing interests.

Additional information

Supplementary Information The online version contains supplementary material available at https://​doi.​org/​

10.​1038/​s41598-​023-​46853-y.

Correspondence and requests for materials should be addressed to T.O.

Reprints and permissions information is available at www.nature.com/reprints.

Publisher’s note Springer Nature remains neutral with regard to jurisdictional claims in published maps and

institutional affiliations.

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